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Extra info for Advances in Chemical Physics, Advancing Theory for Kinetics and Dynamics of Complex, Many-Dimensional Systems: Clusters and Proteins (Volume 145)
The heme ν7 mode was found to be most strongly excited following Q band excitation. By comparing to the deoxy-Mb spectrum, they demonstrated that the signal was derived from 24 hiroshi fujisaki et al. Figure 13. Time course of the ρ11 element of the reduced density matrix for ν4 and ν7 excitations of v = 1. For the explanation of the insets, refer to Ref. 89. (Reproduced with permission from Ref. 86. ) the structural transition from the six-coordinate to the five-coordinate heme. Less prominent excitation of the ν4 mode was also observed.
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